Hi
I am on the road now, so I will have to look up the exact video card tomorrow. But it is a new ATI card and I can load different profiles into the LUT. This seems to work fine.
Yes, the newer ATI cards can handle 3 LUT's providing the software is setup and used correctly. Assuming it is, it sounds like your monitors are very different. It's hard enough to match two monitors of the same type, next would be two different model monitors which support the same gamut, and at the bottom is what you have. Two different models which support different gamuts.
If I was going to attempt this I'd ask myself why. I've used dual monitors for over a decade, two of the exact same monitors side by side on a dual display stand and I love them. Currently I'm using two NEC LCD2690uxi2's.. and using Lightroom or C1 with a dedicated 2nd display monitor is pure luxury. Love it. But with two different monitors I'd ask myself can I set them side by side, do they line up, are they usable as such.. if just for tools and palettes I wouldn't bother profiling the monitor used for tools and palettes.
But if I did.. I'd profile to a gamut which both monitors can handle, which in your case sounds like Srgb. Once I ran through the profiling as close as I could get, then I'd hand/eye tune the white point to get the two as close as possible. And I'd do it realizing they'll never been spot on and it's basically an exercise in futility.. go in not expecting perfection, be pleased if you get something usable.